Dergiler / Hittite Journal of Science and Engineering / 2020 / Cilt: 7 - Sayı: 1

Microwave Assisted Green Synthesis of Ag/AgO Nanocatalyst as An Efficient OER Catalyst in Neutral Media

Sayfa
61–66
Yayın Tarihi
2022-10-18
DOI
—
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⚡ TL;DR(1 Cümlede Hızlı Çıkarım)

The results showed that the developed electrocatalyst system based on Ag/AgO composite could be used in multi-layer electrocatalyst system designs

📌 3 Maddede Bu Makale

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Amaç & Hipotez:T he development of robust, stable and abundant materials that are operating under neutral conditions are of great importance for the electrocatalytic conversion of water to hydrogen using sunlight.
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Temel Bulgular & Veri:The developed Ag/AgO composite catalyst with a small 10-15 nm and homogenous particle size distribution was fabricated using microwave synthesis.
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Sonuç & Katkı:The results showed that the developed electrocatalyst system based on Ag/AgO composite could be used in multi-layer electrocatalyst system designs
🔬Tür:Araştırma Makalesi
📍Kapsam:Genişletilmiş Akademik Örneklem
⚙️Değişkenler:Silver nanoparticles · Microwave · Catalytic activity

Abstract

T he development of robust, stable and abundant materials that are operating under neutral conditions are of great importance for the electrocatalytic conversion of water to hydrogen using sunlight. Here, a robust and highly stable, silver oxide based electrocatalyst composite system for the efficient Oxygen Evolution Reaction OER was presented. The developed Ag/AgO composite catalyst with a small 10-15 nm and homogenous particle size distribution was fabricated using microwave synthesis. In the neutral media, the Ag/AgO electrocatalyst achieved 1 mA cm−2 current density at 600 mV overpotential, and exhibited a lower Tafel slope of 80 mV dec-1 compared to MnOx-based catalysts in the range of 450–600 mV. These values are comparable to those of the promising catalysts such as Mn, Co, Ni oxide based systems in the neutral media. The results showed that the developed electrocatalyst system based on Ag/AgO composite could be used in multi-layer electrocatalyst system designs

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Bu Makaleye Atıf Yap

ELMACI, G. (2022). Microwave Assisted Green Synthesis of Ag/AgO Nanocatalyst as An Efficient OER Catalyst in Neutral Media. Hittite Journal of Science and Engineering, Cilt: 7 - Sayı: 1, 61–66. https://ajindex.com/articles/537947

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Kaynakça (10)

  1. Clark DE, Sutton WH. Microwave processing of materials. Annual Review of Materials Science 26 (1996) 299-331.
  2. Singh S, Gupta D, Jain V, Sharma AK. Microwave processing of materials and applications in manufacturing industries: a review. Materials and Manufacturing Processes 30 (2015) 1-29.
  3. Thostenson E, Chou TW. Microwave processing: fundamentals and applications. Composites Part A: Applied Science and Manufacturing 30 (1999) 1055-1071.
  4. Fan X, Guan J, Li Z, Mou F, Tong G, Wang W. One-pot low temperature solution synthesis, magnetic and microwave electromagnetic properties of single-crystal iron submicron cubes. Journal of Materials Chemistry 20 (2010) 1676-1682.
  5. Cao JM, Feng J, Deng SG, Chang X, Wang J, Liu JS, Lu P, Lu HX, Zheng MB, Zhang F. Microwave-assisted solid-state synthesis of hydroxyapatite nanorods at room temperature. Journal of Materials Science 40 (2005) 6311-6313.
  6. Han Y, Zheng J, Dong E. A novel nonenzymatic hydrogen peroxide sensor based on Ag–MnO2–MWCNTs nanocomposites. Electrochimica Acta 90 (2013) 35-43.
  7. Yang H, Ren Y, Wang T, Wang C. Preparation and antibacterial activities of Ag/Ag+/Ag3+ nanoparticle composites made by pomegranate (Punica granatum) rind extract. Results in physics 6 ( 2016) 299-304. Osterloh F. Inorganic nanostructures for photoelectrochemical and photocatalytic water splitting. Chemical Society Reviews 42 (2013) 2294-2320.
  8. Yi S, Zhang XB, Wulan BR, Yan JM, Jiang Q. Non-noble metals applied to solar water splitting. Energy & Environmental Science 11 (2018) 3128-3156.
  9. Jones MR, Osberg KD, Macfarlane RJ, Langille MR, Mirkin CA. Templated techniques for the synthesis and assembly of plasmonic nanostructures. Chemical Reviews 111 (2011) 3736-3827.
  10. Seh ZW, Kibsgaard J, Dickens CF, Chorkendorff I, Norskov JK, Jaramillo TF. Combining theory and experiment in electrocatalysis: Insights into materials design. Science 355 (2017) eaad4998. Melder J, Kwong WL, Shevela D, Messinger J, Kurz P. Electrocatalytic water oxidation by MnOx /C: In situ catalyst formation, carbon substrate variations, and direct O2/CO2 monitoring by membrane- inlet mass spectrometry. ChemSusChem 10 (2017) 4491-4502.