Dergiler / Turkish Journal of Physics / 2013 / Cilt: 37 - Sayı: 2

The effect of neutron irradiation on the properties of Tl0.6Pb0.3Cd0.1Ba2Ca2Cu3O9-delta superconductors

Sayfa
237–241
DOI
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Özet

The effect of neutron irradiation on phase purity, crystal structure, and electrical resistivity of Tl0.6Pb0.3Cd0.1 Ba2Ca2Cu3O9-delta superconductors has been studied before and after irradiation by electrical resistance measurements and X-ray diffraction techniques. The zero-resistance superconducting transition temperature, Tc(offset), of samples systematically decreases by about 5 K with the increase of neutron irradiation fluence up 18.12 \times 1010 n cm-2. The crystalline phases showed that the compounds have 2 phases, a high-Tc phase (1223) and low-Tc phase (1212), in addition to the impurity phase. The irradiation led to a decrease in oxygen content and volume fraction of high-Tc phase (1223).

Abstract

The effect of neutron irradiation on phase purity, crystal structure, and electrical resistivity of Tl0.6Pb0.3Cd0.1 Ba2Ca2Cu3O9-delta superconductors has been studied before and after irradiation by electrical resistance measurements and X-ray diffraction techniques. The zero-resistance superconducting transition temperature, Tc(offset), of samples systematically decreases by about 5 K with the increase of neutron irradiation fluence up 18.12 \times 1010 n cm-2. The crystalline phases showed that the compounds have 2 phases, a high-Tc phase (1223) and low-Tc phase (1212), in addition to the impurity phase. The irradiation led to a decrease in oxygen content and volume fraction of high-Tc phase (1223).

Anahtar kelimeler: Irradiation, superconductors, crystal structure, X-ray diffraction, resistivity, Tc