Journals / Atmospheric Pollution Research / 2016 / Cilt: 7 - Sayı: 6

Pollution characteristics of atmospheric particulate mercury near a coal-fired power plant on the southeast coast of China

Pages
1119–1127
DOI
—
🏛️Bibliographic metadata and full text access for this article are provided via DergiPark.
DergiPark Record ↗
✨

AI Summary & Key Takeaways

AI Insight
⚡ TL;DR(Too Long; Didn't Read)

In contrast to RPM, the percentageof both HPM and EPM in PM2.5 was higher than in PM10.

📌 3 Key Takeaways

🎯
Objective & Hypothesis:PM2.5 and PM10 samples were collected in a rural area from December 2014 to August 2015 near a coalfiredpower plant on the southeast coast of China.
📊
Key Findings & Data:The total mercury concentrations in PM2.5 ranged from116.2 to 1070.9 pg/m3 and in PM10 from 173.4 to 1456.8 pg/m3, with averages of 309.5 ± 94.9 and387.5 ± 133.5 pg/m3, respectively.
💡
Conclusion & Impact:In contrast to RPM, the percentageof both HPM and EPM in PM2.5 was higher than in PM10.
🔬Design:Research Article
📍Scope:2014 · 10 samples
⚙️Variables:Domain Parameters

Özet

PM2.5 and PM10 samples were collected in a rural area from December 2014 to August 2015 near a coalfiredpower plant on the southeast coast of China. The total mercury concentrations in PM2.5 ranged from116.2 to 1070.9 pg/m3 and in PM10 from 173.4 to 1456.8 pg/m3, with averages of 309.5 ± 94.9 and387.5 ± 133.5 pg/m3, respectively. These were much higher than those found in many foreign cities. Theconcentrations of mercury in PM2.5 and PM10 varied seasonally, with the highest average concentrationin winter. This was probably due to the seasonal variation of meteorological conditions and concentrationof particulates. The highest mass-based concentration of mercury in PM2.5 and PM10 was observed inspring. This result might be related to the prevailing sea winds in spring. The spatial variation of particulatemercury conformed to the concentration distribution characteristics of pollutant dischargedfrom coal-fired power plant elevated source at the downwind area. The seasonal variation in the concentrationsof the four mercury species (including exchangeable particulate mercury: EXPM, HCl-solubleparticulate mercury: HPM, elemental particulate mercury: EPM, and residual particulate mercury: RPM)were all identical to the seasonal variation of total particulate mercury (TPM) in PM2.5 and PM10(winter > spring > summer). Owing to the variation of meteorological conditions, the proportion ofdifferent mercury species in TPM followed different seasonal trends. In contrast to RPM, the percentageof both HPM and EPM in PM2.5 was higher than in PM10.

🔖

Cite This Article

GAO, J., WANG, H., CAI, W., WU, J., HE, Y. (2016). Pollution characteristics of atmospheric particulate mercury near a coal-fired power plant on the southeast coast of China. Atmospheric Pollution Research, Cilt: 7 - Sayı: 6, 1119–1127. https://ajindex.com/articles/351522

References (1)

  1. AMAP/UNEP, 2013. Technical Background Report for the Global Mercury Assessment 2013. Arctic Monitoring and Assessment Programme, Oslo, Norway/UNEP Chemicals Branch, Geneva, Switzerland. Ames, M., Gullu, G., Olmez, I., 1998. Atmospheric mercury in the vapor phase, and in fine and coarse particulate matter at Perch River, New York. Atmos. Environ. 32, 865e872. Brooks, S., Luke, W., Cohen, M., Kelly, P., Lefer, B., Rappenglück, B., 2010. Mercury species measured atop the Moody Tower TRAMP site, Houston, Texas. Atmos. Environ. 44, 4045e4055. Cao, J.J., Lee, S.C., Ho, K.F., Zhang, X.Y., Zou, S.C., Fung, K., Chow, J.C., Watson, J.G., 2003. Characteristics of carbonaceous aerosol in Pearl river Delta region, China during 2001 winter period. Atmos. Environ. 37, 1451e1460. Clarke, L.B., 1993. The fate of trace elements during coal combustion and gasification: an overview. Fuel 72, 731e736. Eckley, C.S., Gustin, M., Miller, M.B., Marsik, F., 2011. Scaling non-point-source mercury emissions from two active industrial gold mines: influential variables and annual emission estimates. Environ. Sci. Technol. 45, 392e399. Engle, M.A., Gustin, M.S., 2002. Scaling of atmospheric mercury emissions from three naturally enriched areas: Flowery Peak, Nevada; Peavine Peak, Nevada; and Long Valley Caldera, California. Sci. Total Environ. 290, 91e104. Fang, F.M., Wang, Q.C., Li, J.F., 2001. Atmospheric particulate mercury concentration and its dry deposition flux in Changchun City, China. Sci. Total Environ. 281, 229e236. Fitzgerald, W.F., Engstrom, D.R., Mason, R.P., Nater, E.A., 1998. The case for atmospheric mercury contamination in remote areas. Environ. Sci. Technol. 32, 1e7. Fu, X.W., Feng, X.B., Qiu, G.L., Shang, L.H., Zhang, H., 2011. Speciated atmospheric mercury and its potential source in Guiyang, China. Atmos. Environ. 45, 4205e4212. Gbor, P.K., Wen, D., Meng, F., Yang, F., Sloan, J.J., 2007. Modeling of mercury emission, transport and deposition in North America. Atmos. Environ. 41, 1135e1149. Gildemeister, A.E., Graney, J., Keeler, G.J., 2005. Source proximity reflected in spatial and temporal variability in particle and vapor phase Hg concentrations in Detroit, MI. Atmos. Environ. 39, 353e358. Hall, B., 1995. The gas phase oxidation of elemental mercury by ozone. Water Air Soil Pollut. 80, 301e315. Jiang, G.B., Shi, J.B., Feng, X.B., 2006. Mercury pollution in China. An overview of the past and current sources of the toxic metal. Environ. Sci. Technol. 40. Keeler, G.