Journals / Atmospheric Pollution Research / 2019 / Cilt: 10 - Sayı: 5

Pollution characteristics and risk assessment of ambient PM2.5-bound PAHs and NPAHs in typical Japanese and New Zealand cities and rural sites

Pages
1396–1403
DOI
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AI Summary & Key Takeaways

AI Insight
⚡ TL;DR(Too Long; Didn't Read)

Back trajectory analyses showed that high levels of PAHs detected at Wajima were theresult of long-range transport from China and Mongolia in winter, which was not observed at the other sites.Considering the adverse health effects of PM2.5, further studies and continuous monitoring of atmospheric PAHsand NPAHs are necessary to evaluate mitigation strategies in both hemispheres.

📌 3 Key Takeaways

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Objective & Hypothesis:Nine polycyclic aromatic hydrocarbons (PAHs) and six nitro-PAHs (NPAHs) were measured in PM2.5 samplescollected over one year (2016–2017) in two cities: Kanazawa (Japan) and Auckland (New Zealand) and theirrespective rural background sites: Wajima in Noto Peninsula (Japan) and Tapora in Okahukura Peninsula (NewZealand).
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Key Findings & Data:The mean of ΣPAHs in Kanazawa City was0.53 ng/m3 and represented the highest total concentration compared to the other three sites.
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Conclusion & Impact:Back trajectory analyses showed that high levels of PAHs detected at Wajima were theresult of long-range transport from China and Mongolia in winter, which was not observed at the other sites.Considering the adverse health effects of PM2.5, further studies and continuous monitoring of atmospheric PAHsand NPAHs are necessary to evaluate mitigation strategies in both hemispheres.
🔬Design:Research Article
📍Scope:2016–2017 · 2.5 samples
⚙️Variables:Domain Parameters

Özet

Nine polycyclic aromatic hydrocarbons (PAHs) and six nitro-PAHs (NPAHs) were measured in PM2.5 samplescollected over one year (2016–2017) in two cities: Kanazawa (Japan) and Auckland (New Zealand) and theirrespective rural background sites: Wajima in Noto Peninsula (Japan) and Tapora in Okahukura Peninsula (NewZealand). The mean concentrations of ΣPAHs and ΣNPAHs followed similar distribution profiles in both countries,with higher concentrations in the urban than rural sites. The mean of ΣPAHs in Kanazawa City was0.53 ng/m3 and represented the highest total concentration compared to the other three sites. Conversely, thehighest ΣNPAHs concentrations were measured in Auckland City (48.2 pg/m3). Diagnostic ratios and principalcomponent analysis revealed that automobiles were the main sources of PAHs and NPAHs in both cities, whereascoal combustion and domestic wood burning were the dominant sources of PAHs and NPAHs in rural sites inJapan and New Zealand. Back trajectory analyses showed that high levels of PAHs detected at Wajima were theresult of long-range transport from China and Mongolia in winter, which was not observed at the other sites.Considering the adverse health effects of PM2.5, further studies and continuous monitoring of atmospheric PAHsand NPAHs are necessary to evaluate mitigation strategies in both hemispheres.

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Cite This Article

KALİSA, E., NAGATO, E., BİZURU, E., LEE, K., TANG, N., POİNTİNG, S., HAYAKAWA, K., ARCHER, S., BUGLER, D. L. (2019). Pollution characteristics and risk assessment of ambient PM2.5-bound PAHs and NPAHs in typical Japanese and New Zealand cities and rural sites. Atmospheric Pollution Research, Cilt: 10 - Sayı: 5, 1396–1403. https://ajindex.com/articles/351453

References (9)

  1. Abdel-Shafy, H.I., Mansour, M.S., 2016. A review on polycyclic aromatic hydrocarbons: source, environmental impact, effect on human health and remediation. Egypt. J. Petrol. 25 (1), 107–123.
  2. Alam, M.S., Keyte, I.J., Yin, J., Stark, C., Jones, A.M., Harrison, R.M., 2015. Diurnal variability of polycyclic aromatic compound (PAC) concentrations: relationship with meteorological conditions and inferred sources. Atmos. Environ. 122, 427–438.
  3. Albinet, A., Leoz-Garziandia, E., Budzinski, H., Villenave, E., Jaffrezo, J.L., 2008. Nitrated and oxygenated derivatives of polycyclic aromatic hydrocarbons in the ambient air of two French alpine valleys: Part 1: concentrations, sources and gas/particle partitioning. Atmos. Environ. 42 (1), 43–54. Amador-Muñoz, O., Villalobos-Pietrini, R., Miranda, J., Vera-Avila, L.E., 2011. Organic compounds of PM2.5 in Mexico Valley: spatial and temporal patterns, behavior and sources. Sci. Total Environ. 409 (8), 1453–1465.
  4. Atkinson, R., Arey, J., 1994. Atmospheric chemistry of gas-phase polycyclic aromatic hydrocarbons: formation of atmospheric mutagens. Environ. Health Perspect. 102, 117–126.
  5. Bamford, H.A., Baker, J.E., 2003. Nitro-polycyclic aromatic hydrocarbon concentrations and sources in urban and suburban atmospheres of the Mid-Atlantic region. Atmos. Environ. 37 (15), 2077–2091.
  6. Bandowe, B.A.M., Meusel, H., Huang, R.J., Ho, K., Cao, J., Hoffmann, T., Wilcke, W., 2014. PM2.5-bound oxygenated PAHs, nitro-PAHs and parent-PAHs from the atmosphere of a Chinese megacity: seasonal variation, sources and cancer risk assessment. Sci. Total Environ. 473, 77–87.
  7. Bari, M.A., Baumbach, G., Kuch, B., Scheffknecht, G., 2010. Particle-phase concentrations of polycyclic aromatic hydrocarbons in ambient air of rural residential areas in southern Germany. Air Qual. Atmos. Heal. 3 (2), 103–116. Błaszczyk, E., Rogula-Kozłowska, W., Klejnowski, K., Fulara, I., Mielżyńska-Švach, D., 2017. Polycyclic aromatic hydrocarbons bound to outdoor and indoor airborne particles (PM2. 5) and their mutagenicity and carcinogenicity in Silesian kindergartens, Poland. Air Qual. Atmos. Hlth. 10 (3), 389–400.
  8. Boström, C.E., Gerde, P., Hanberg, A., Jernström, B., Johansson, C., Kyrklund, T., Westerholm, R., 2002. Cancer risk assessment, indicators, and guidelines for polycyclic aromatic hydrocarbons in the ambient air. Environ. Health Perspect. 110, 451–489.
  9. Brown, L.E., Trought, K.R., Bailey, C.I., Clemons, J.H., 2005. 2, 3, 7, 8-TCDD equivalence and mutagenic activ