Journals / Atmospheric Pollution Research / 2020 / Cilt: 11 - Sayı: 11

Seasonal characteristics of PM2.5 and its chemical species in the northern rural China

Pages
1891–1901
DOI
—
🏛️Bibliographic metadata and full text access for this article are provided via DergiPark.
DergiPark Record ↗
✨

AI Summary & Key Takeaways

AI Insight
⚡ TL;DR(Too Long; Didn't Read)

Strong variations ofPM2.5 and its species above on a timescale of seasons indicated that the local sources, such as coal combustionand biomass burning, dominated the local atmospheric pollutants.

📌 3 Key Takeaways

🎯
Objective & Hypothesis:Daily PM2.5 samples were collected at a rural site in North China for four consecutive seasons from summer of2015 to spring of 2016.
📊
Key Findings & Data:Results revealed that the studied rural area suffered from severe PM2.5 pollution with itsannual average concentration of 109.6 ± 45.0 μg m−3, which was about 3.1 times higher than the national airquality standard of China.
💡
Conclusion & Impact:Strong variations ofPM2.5 and its species above on a timescale of seasons indicated that the local sources, such as coal combustionand biomass burning, dominated the local atmospheric pollutants.
🔬Design:Research Article
📍Scope:2016 · 2.5 samples
⚙️Variables:Domain Parameters

Özet

Daily PM2.5 samples were collected at a rural site in North China for four consecutive seasons from summer of2015 to spring of 2016. Results revealed that the studied rural area suffered from severe PM2.5 pollution with itsannual average concentration of 109.6 ± 45.0 μg m−3, which was about 3.1 times higher than the national airquality standard of China. Among all identified species, water soluble inorganic ions (WSIIs) were the majorcomponent, accounting for 46.0 ± 11.1% of PM2.5 mass. The sum of element carbon (EC) and organic carbon(OC) accounting for 24.1 ± 11.5%. The trace elements accounted for about only 2% of PM2.5 mass. The resultsof the chemical mass balance of PM2.5 showed that 74–99% of the PM2.5 mass can be reconstructed by theidentified species. SNA (the sum of SO42−, NO3− and NH4+) and particulate organic matter (POM) were evidenttwo kinds of predominant components of the PM2.5, which together accounted for ~60%, with seasonal variations. Mineral dust and EC accounted for ~8% and ~7%, respectively. The trace element oxide (TEO), biomassburning-derived K+ and coal combustion-derived Cl− together represented about 10%. Strong variations ofPM2.5 and its species above on a timescale of seasons indicated that the local sources, such as coal combustionand biomass burning, dominated the local atmospheric pollutants.

🔖

Cite This Article

LIU, K., REN, J. (2020). Seasonal characteristics of PM2.5 and its chemical species in the northern rural China. Atmospheric Pollution Research, Cilt: 11 - Sayı: 11, 1891–1901. https://ajindex.com/articles/351317

References (8)

  1. Bealey, W.J., McDonald, A.G., Nemitz, E., Donovan, R., Dragosits, U., Duffy, T.R., Fowler, D., 2007. Estimating the reduction of urban PM10 concentrations by trees within an environmental information system for planners. J. Environ. Manag. 85, 44–58.
  2. Bhuyan, P., Deka, P., Prakash, A., Balachandran, S., Hoque, R.R., 2018. Chemical characterization and source apportionment of aerosol over mid Brahmaputra Valley, India. Environ. Pollut. 234, 997–1010. Bläsing, M., Müller, M., 2012. Release of alkali metal, sulfur, and chlorine species during high-temperature gasification of coal and coal blends in a drop tube reactor. Energy Fuel. 26, 6311–6315.
  3. Buseck, P.R., Posfai, M., 1999. Airborne minerals and related aerosol particles: effects on climate and the environment. Proc. Natl. Acad. Sci. U. S. A. 96, 3372–3379.
  4. Cao, J.J., Lee, S.C., Chow, J.C., Watson, J.G., Ho, K.F., Zhang, R.J., Jin, Z.D., Shen, Z.X., Chen, G.C., Kang, Y.M., Zou, S.C., Zhang, L.Z., Qi, S.F., Dai, M.H., Cheng, Y., Hu, K., 2007. Spatial and seasonal distributions of carbonaceous aerosols over China. J. Geophys. Res. 112, D22S11. Castro, L.M., Pio, C.A., Harrison, R.M., Smith, D.J.T., 1999. Carbonaceous aerosol in urban and rural European atmospheres_ Estimation of secondary organic carbon concentrations. Atmos. Environ. 33, 2771–2781.
  5. Chen, D., Cui, H., Zhao, Y., Yin, L., Lu, Y., Wang, Q., 2017a. A two-year study of carbonaceous aerosols in ambient PM2.5 at a regional background site for western Yangtze River Delta, China. Atmos. Res. 183, 351–361.
  6. Chen, G., Zhang, W., Li, S., Zhang, Y., Williams, G., Huxley, R., Ren, H., Cao, W., Guo, Y., 2017b. The impact of ambient fine particles on influenza transmission and the modification effects of temperature in China: a multi-city study. Environ. Int. 98, 82–88.
  7. Cheng, Y., Engling, G., He, K.B., Duan, F.K., Ma, Y.L., Du, Z.Y., Liu, J.M., Zheng, M., Weber, R.J., 2013. Biomass burning contribution to Beijing aerosol. Atmos. Chem. Phys. 13, 7765–7781.
  8. Cheng, Y.F., Eichler, H., Wiedensohler, A., Heintzenberg, J., Zhang, Y.H., Hu, M., Herrmann, H., Zeng, L.M., Liu, S., Gnauk, T., Brüggemann, E., He, L.Y., 2006. Mixing state of elemental carbon and non-light-absorbing aerosol components derived from in situ particle optical properties at Xinken in Pearl River Delta of China. J. Geophys. Res. 111. Fan, K., Xie, Z., Wang, H., Xu, Z., Liu, J., 2018. Frequency of spring dust weather in North China linked to sea ice variability in the Barents Sea. Clim. Dynam.